A few schools require FAFSA for non-need-based merit scholarships, typically to rule out Pell eligibility before awarding a giant scholarship. Emphasis on "few!" Other than that, typically most requirements for financial aid forms involve a need component for the scholarship. Check the scholarship webpages for the colleges in question.
CSS Profile is a different beast. I don't believe any require the CSS Profile for non-need-based merit, though obviously I don't know all possible exceptions, so again, check scholarship websites for colleges.